The purpose of this study is to provide insights into the neutronic similarities that may exist between a
generic cask containing typical spent nuclear fuel assemblies and commercial reactor critical (CRC) state-
points. Forty CRC state-points from five pressurized-water reactors were selected for the study and the
type of CRC state-points that may be applicable for validation of burnup credit criticality safety
calculations for spent fuel transport/storage/disposal systems are identified. The study employed cross-

This report presents the results of computer code benchmark simulations against spent fuel radiochemical assay
measurements from the Kansai Electric Ltd. Takahama-3 reactor published by the Japan Atomic Energy
Research Institute. Takahama-3 is a pressurized-water reactor that operates with a 17 × 17 fuel-assembly design.
Spent fuel samples were obtained from assemblies operated for 2 and 3 cycles and achieved a maximum burnup
of 47 GWd/MTU. Radiochemical analyses were performed on two rods having an initial enrichment of

Uncertainties in the predicted isotopic concentrations in spent nuclear fuel represent one of the largest
sources of overall uncertainty in criticality calculations that use burnup credit. The methods used to
propagate the uncertainties in the calculated nuclide concentrations to the uncertainty in the predicted
neutron multiplication factor (keff) of the system can have a significant effect on the uncertainty in the
safety margin in criticality calculations and ultimately affect the potential capacity of spent fuel transport

This paper provides insights into the neutronic similarities between a representative high-capacity rail-transport cask containing typical pressurized water reactor (PWR) spent nuclear fuel assemblies and critical reactor state-points, referred to as commercial reactor critical (CRC) state-points. Forty CRC state-points from five PWRs were analyzed, and the characteristics of CRC state-points that may be applicable for validation of burnup-credit criticality safety calculations for spent fuel transport/storage/disposal systems were identified.

This report presents a methodology for validation of the isotopic
contents of spent light water reactor fuel for actinide-only burnup
credit with additional high-quality radiochemistry assay (RCA) data
obtained from the Yankee Rowe pressurized water reactor. The
additional Yankee Rowe RCA data were not included in previous
isotopic validation studies for burnup credit due to the difficulty of
accurately modeling the complex Yankee Rowe fuel assembly design
using the SAS2H one-dimensional sequence of the earlier SCALE

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

This report is part of a report series designed to document benchmark-quality radiochemical isotopic
assay data against which computer code accuracy can be quantified to establish the uncertainty and bias
associated with the code predictions. The experimental data included in the report series were acquired
from domestic and international programs and include spent fuel samples that cover a large burnup range.
The measurements analyzed in the current report, for which experimental data is publicly available,