This report is part of a report series designed to document benchmark-quality radiochemical assay data
against which computer code predictions of isotopic composition for spent nuclear fuel can be validated
to establish the uncertainty and bias associated with the code predictions. The experimental data analyzed
in the present report were acquired from two international programs: (1) ARIANE and (2) REBUS, both
coordinated by Belgonucleaire. All measurements include extensive actinide and fission product data of

The results of an extensive update of the decay data of the ORIGEN-S library are presented
in this report. The updated decay data were provided for both the ORIGEN-S and ORIGEN2
libraries in the same project. A complete edit of the decay data plus the available half-life
uncertainties are included in Appendix A. A detailed description of the types of data contained in the
library, the format of the library, and the data sources are also presented. Approximately 24% of the

The purpose of this calculation is to perform an example criticality evaluation for degraded internal configurations of a boiling water reactor (BWR) waste package (WP) containing 44 spent nuclear fuel (SNF) assemblies. The BWR assembly design considered is based on the General Electric (GE) 8x8 assembly (see section 5.1). Depletion analyses for various assembly average enrichment and burnup (expressed as gigawatt days/metric ton Uranium; GWd/MTU) combinations are performed using the SAS2H/ORIGEN-S sequence of SCALE 4.3 (CSCI:30011-2002; Ref. 7.5).