The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.