This report presents a methodology for validation of the isotopic
contents of spent light water reactor fuel for actinide-only burnup
credit with additional high-quality radiochemistry assay (RCA) data
obtained from the Yankee Rowe pressurized water reactor. The
additional Yankee Rowe RCA data were not included in previous
isotopic validation studies for burnup credit due to the difficulty of
accurately modeling the complex Yankee Rowe fuel assembly design
using the SAS2H one-dimensional sequence of the earlier SCALE

This research examines the practice of equating the reactivity of spent fuel to that of fresh fuel for the purpose of performing burnup credit criticality safety analyses for PWR spent fuel pool (SFP) storage conditions. The investigation consists of comparing kf estimates based on reactivity "equivalent" fresh fuel enrichment (REFFE) to kl estimates using the actual spent fuel isotopics.

The concept of direct disposal of dual-purpose canisters (DPCs) has not been previously considered
for the Yucca Mountain geologic repository because of concerns, among other reasons,
about degradation of the reactivity-control material over the relatively long period of the repository
analyses. Aluminum-based neutron absorber materials, typically used in DPCs, are not
expected to have sufficient corrosion resistance necessary to retain their integrity over a 10,000+

Analytical methods, described in this report, are used to
systematically determine experimental fuel sub-batch
reactivities as a function of burnup. Fuel sub-batch reactivities
are inferred using more than 600 in-core pressurized water
reactor (PWR) flux maps taken during 44 cycles of operation
at the Catawba and McGuire nuclear power plants. The
analytical methods systematically search for fuel sub-batch
reactivities that minimize differences between measured and
computed reaction rates, using Studsvik Scandpower’s

Until now, the Nuclear Regulatory Commission's (NRC) approval of criticality safety evaluations for spent fuel in transport and storage casks has been based on analyzing the fuel as though it were fresh and without burnable poisons. The well-known nuclide composition of fresh fuel has provided a straightforward and bounding approach for showing that spent fuel systems will remain subcritical under normal and accident conditions. Burnup credit refers to the approval of criticality safety evaluations that consider the decrease in fuel reactivity caused by. irradiation in the reactor.

Criticality safety analysis devoted to spent-fuel storage and transportation has to be conservative in order to be sure no accident will ever happen. In the spent-fuel storage field, the assumption of freshness has been used to achieve the conservative aspect of criticality safety procedures. Nevertheless, after being irradiated in a reactor core, the fuel elements have obviously lost part of their original reactivity. The concept of taking into account this reactivity loss in criticality safety analysis is known as burnup credit.