This report presents a methodology for validation of the isotopic
contents of spent light water reactor fuel for actinide-only burnup
credit with additional high-quality radiochemistry assay (RCA) data
obtained from the Yankee Rowe pressurized water reactor. The
additional Yankee Rowe RCA data were not included in previous
isotopic validation studies for burnup credit due to the difficulty of
accurately modeling the complex Yankee Rowe fuel assembly design
using the SAS2H one-dimensional sequence of the earlier SCALE

A flat, uniform axial burnup assumption, preferred for its computational simplicity, does not always conservatively estimate the pressurized water reactor spent-fuel-cask multiplication factors. Rather, the reactivity effect of the significantly underburned fuel ends, usually referred to as the "end effect," can be properly treated by explicit modeling of the axial burnup distribution based on limiting axial burnup profiles.

In the 1980s a series of the Haut Taux de Combustion (HTC) critical experiments with fuel pins in a water-moderated lattice was conducted at the Apparatus B experimental facility in Valduc (Commissariat à l'Energie Atomique, France) with the support of the Institut de Radioprotection et de Sûreté Nucléaire and AREVA NC. Four series of experiments were designed to assess profit associated with actinide-only burnup credit in the criticality safety evaluation for fuel handling, pool storage, and spent-fuel cask conditions.

In the 1980s, a series of critical experiments referred to as the Haut Taux de Combustion (HTC)
experiments was conducted by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) at the
experimental criticality facility in Valduc, France. The plutonium-to- uranium ratio and the isotopic
compositions of both the uranium and plutonium used in the simulated fuel rods were designed to be
similar to what would be found in a typical pressurized-water reactor fuel assembly that initially had an

This report describes a novel approach developed at the Oak Ridge National Laboratory
(ORNL) for the estimation of the uncertainty in the prediction of the neutron multiplication factor
for spent nuclear fuel. This technique focuses on burnup credit, where credit is taken in criticality
safety analysis for the reduced reactivity of fuel irradiated in and discharged from a reactor.
Validation methods for burnup credit have attempted to separate the uncertainty associated with

The objective of this calculation is to provide the uncertainty term for fission product and minor actinides which contributes to the determination of the critical limit for burnup credit calculations. The scope of this calculation covers PWR and BWR spent nuclear fuel. This activity supports the Criticality Department's validation of burnup credit. The intended use of these results is in future Criticality Department calculations and analyses.