Disposal Criticality Analysis Methodology Topical Report describes a methodology for performing postclosure criticality analyses within the repository at Yucca Mountain, Nevada. An important component of the postclosure criticality analysis is the calculation of conservative isotopic concentrations for spent nuclear fuel. This report documents the isotopic calculation methodology. The isotopic calculation methodology is shown to be conservative based upon current data for pressurized water reactor and boiling water reactor spent nuclear fuel.

The objective of the Limerick Unit 1 Radiochemical Assay Comparisons to SAS2H Calculations is to determine the accuracy of the SAS2H control module of the baselined modular code system SCALE, Version 4.4A (STN: 10129-4.4A-00), in predicting the isotopic concentrations of spent fuel, and to quantify the overall effect that the differences between the calculated and measured isotopic concentrations have on the system reactivity. The scope of this calculation covers eight different spent fuel samples from a fuel assembly that was irradiated in the Limerick Unit 1 boiling water reactor (BWR).

As part of a larger program to study mixed-oxide fuel subject to high burnup, some UO2 samples were exposed and analyzed. This report discusses results from the analysis of a UO sample that was burned in a boiling-water reactor (BWR) to approximately 57 GWd/t. The sample

The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.

The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

This calculation file provides comparisons of one- and two-dimensional methods for calculating the isotopic content of spent nuclear fuel. The one-dimensional methods use the SAS2H sequence of SCALE 4.4a (Reference 7.1) and the SAS2 sequence of SCALE 5.0 (Reference 7.2). The two-dimensional method uses the TRITON control module along with the T-DEPL sequence of SCALE 5.0 (Reference 7.3). The SAS2H results for SCALE 4.4a are taken from Reference 7.4. Data from previous two-dimensional calculations (Reference 7.5) using CASM03 will also be used for comparisons with TRITON.

This calculation demonstrates how uncertainties in half-life and branching fraction affect postclosure isotopic concentrations and the quantification of those effects in terms of reactivity.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

This calculation compares results from criticality evaluations for a 21-assembly pressurized water reactor (PWR) waste package based on 12 axial burnup profile representations for commercial spent nuclear fuel (SNF) assemblies. The burnup profiles encompass the axial variations caused by different fuel assembly irradiation histories in a commercial PWR, including end effects, and the concomitant effect on reactivity in the waste package. The bounding axial burnup profiles in Table T of reference 6.3 are used for this analysis.