The purpose of this calculation is to perform intact mode and partially degraded mode criticality evaluations of the Department of Energy's (DOE) Enrico Fermi (EF) Spent Nuclear Fuel (SNF) co-disposed in a 5 Defense High-Level Waste (5-DHLW) Waste Package (WP) and emplaced in a Monitored Geologic Repository (MGR). The criticality evaluations estimate the values of the effective neutron multiplication factor, keff, as a measure of nuclear criticality potential, for the 5- DHLW/DOE SNF WP with intact or partially degraded internal configurations.

There are more than 250 forms of U.S. Department of Energy (DOE)-owned spent nuclear fuel (SNF). Due to the variety of the spent nuclear fuel, the National Spent Nuclear Fuel Program (NSNFP) has designated nine representative fuel groups for disposal criticality analyses based on fuel matrix, primary fissile isotope, and enrichment. Fast Flux Test Facility (FFTF) fuel has been designated as the representative fuel for the mixed-oxide (MOX) fuel group which is a mixture of uranium and plutonium oxides.

This report is developed from Technical Work Plan for: Thermodynamic Databases for Chemical Modeling (BSC 2006 [DIRS 177885]). The purpose of this analysis report is to update the thermochemical database data0.ymp.R4 (Output DTN: SN0410T0510404.002). Various data have been added, corrected, or corroborated, partly in response to four Condition Reports (CRs): CR 6489, CR 6731, CR 7542, and CR 7756. The most notable changes are a general revision of phosphate data to achieve consistency with the recommendations from the Committee on Data for Science and Technology (CODATA) (Cox. et al.

This analysis is prepared by the Mined Geologic Disposal System (MGDS) Waste Package Development (WPD) department to provide an evaluation of the criticality potential within a waste package having some or all of its contents degraded by corrosion and removal of neutron absorbers. This analysis is also intended to provide an estimate of the consequences of any internal criticality, particularly in terms of any increase in radionuclide inventory. These consequence estimates will be used as part of the WPD input to the Total System Performance Assessment.

The purpose of this calculation is to perform the same reactivity calculations as performed in Reference 7.1 and Reference 7.2 for a set of Laboratory Critical Experiments (LCE) except to change some of the cross section libraries as specified here, and to perform sixteen additional calculations for U233 LCEs.

The purpose of this calculation is to establish the relative change in the effective neutron multiplication factor (keff) due to the use of MCNP unique identifiers (ZAIDs) in Nuclear Criticality Calculations for Canister-Based Facilities - DOE SNF (Reference 2.2.1, Attachment 3, MCNP inputs.zip) that are different to the ZAIDs used in the Analysis of Critical Benchmark Experiments and Critical Limit Calculation for DOE SNF (Reference 2.2.5, Table 5-3).

The purpose of this analysis is to evaluate the types of defects or imperfections that could occur in a waste package or a drip shield and potentially lead to its early failure, and to estimate a probability of undetected occurrence for each type. An early failure is defined as the through-wall penetration of a waste package or drip shield due to manufacturing or handling-induced defects, at a time earlier than would be predicted by mechanistic degradation models for a defect-free waste package or drip shield.

The purpose of this calculation is to perform criticality evaluations for mixed oxide spent nuclear fuel (MOX SNF) in 12 and 21 Pressurized Water Reactor (PWR) waste packages (WPs) for both intact and degraded configurations.
The MOX assembly design considered in previous studies on Pu disposition in commercial reactors is based on the Westinghouse (W) 17x17 Vantage 5 assembly (Ref. 7.2). Depletion analyses of four Pu enrichment and burnup (expressed as gigawatt days/metric ton heavy metal; GWd/MTHM) combinations were performed in Reference 7.4. These are:

The means to prevent and control criticality must be addressed as part of the Preclosure Safety Analysis (PCSA) required for compliance with 10 CFR Part 63 [DIRS 180319], where the preclosure period covers the time prior to permanent closure activities. This technical report presents the nuclear criticality safety evaluation that documents the achievement of this objective.