The purpose of this calculation is to develop an estimate of the isotopic content as a function of time for mixed oxide (MOX) spent nuclear fuel (SNF) assemblies in a Westinghouse pressurized water reactor (PWR). These data will be used as source data for criticality, thermal, and radiation shielding evaluations of waste package (WP) designs for MOX assemblies in the Monitored Geologic Repository (MGR).

The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

This analysis is prepared by the Mined Geologic Disposal System (MODS) Waste Package Development (WPD) department to provide an evaluation of the criticality potential within a waste package having some or all of its contents degraded by corrosion and removal of neutron absorbers. This analysis is also intended to provide an estimate of the consequences of any internal criticality, particularly in terms of any increase in radionuclide inventory. These consequence estimates will be used as part of the WPD input to the Total System Performance Assessment.

This analysis is prepared by the Mined Geologic Disposal System (MGDS) Waste Package Development (WPD) department to provide a probabilistic evaluation of the potential for criticality of fissile material which has been transported from a geologic repository containing breached waste packages of commercial spent nuclear fuel (SNF). This analysis is part of a continuing investigation of the probability of criticality resulting from the emplacement of spent nuclear fuel in a geologic repository.

The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

The purpose of this analysis is to provide an initial radionuclide inventory (in grams per waste package) and associated uncertainty distributions for use in the Total System Performance Assessment for the License Application (TSPA-LA) in support of the license application for the repository at Yucca Mountain, Nevada. This document is intended for use in postclosure analysis only.

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

This paper provides insights into the neutronic similarities between a representative high-capacity rail-transport cask containing typical pressurized water reactor (PWR) spent nuclear fuel assemblies and critical reactor state-points, referred to as commercial reactor critical (CRC) state-points. Forty CRC state-points from five PWRs were analyzed, and the characteristics of CRC state-points that may be applicable for validation of burnup-credit criticality safety calculations for spent fuel transport/storage/disposal systems were identified.

In the 1980s a series of the Haut Taux de Combustion (HTC) critical experiments with fuel pins in a water-moderated lattice was conducted at the Apparatus B experimental facility in Valduc (Commissariat à l'Energie Atomique, France) with the support of the Institut de Radioprotection et de Sûreté Nucléaire and AREVA NC. Four series of experiments were designed to assess profit associated with actinide-only burnup credit in the criticality safety evaluation for fuel handling, pool storage, and spent-fuel cask conditions.

The objective of this calculation is to establish an isotopic database to represent commercial spent nuclear fuel (CSNF) from boiling water reactors (BWRs) in criticality analyses performed for the proposed Monitored Geologic Repository at Yucca Mountain, Nevada. Confirmation of the conservatism with respect to criticality in the isotopic concentration values represented by this isotopic database is performed as described in Section 3.5.3.1.2 of the Disposal Criticality Analysis Methodology Topical Report (Reference 7.1).

The purpose of this calculation report, Range of Applicability and Bias Determination for Postclosure
Criticality of Commercial Spent Nuclear Fuel, is to validate the computational method used to perform
postclosure criticality calculations. The validation process applies the criticality analysis methodology
approach documented in Section 3.5 of the Disposal Criticality Analysis Methodology Topical Report.1
The application systems for this validation consist of waste packages containing transport, aging, and

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

The purpose of this report is to document and validate the external accumulation model that predicts accumulation of fissile materials in the invert, fractures and lithophysae in the rock beneath a degrading waste package containing spent nuclear fuel (SNF) in the monitored geologic repository at Yucca Mountain. (Lithophysae are hollow, bubblelike structures in the rock composed of concentric shells of finely crystalline alkali feldspar, quartz, and other materials (Bates and Jackson 1984 [DIRS 128109], p.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

This calculation file provides comparisons of one- and two-dimensional methods for calculating the isotopic content of spent nuclear fuel. The one-dimensional methods use the SAS2H sequence of SCALE 4.4a (Reference 7.1) and the SAS2 sequence of SCALE 5.0 (Reference 7.2). The two-dimensional method uses the TRITON control module along with the T-DEPL sequence of SCALE 5.0 (Reference 7.3). The SAS2H results for SCALE 4.4a are taken from Reference 7.4. Data from previous two-dimensional calculations (Reference 7.5) using CASM03 will also be used for comparisons with TRITON.

Disposal Criticality Analysis Methodology Topical Report describes a methodology for performing postclosure criticality analyses within the repository at Yucca Mountain, Nevada. An important component of the postclosure criticality analysis is the calculation of conservative isotopic concentrations for spent nuclear fuel. This report documents the isotopic calculation methodology. The isotopic calculation methodology is shown to be conservative based upon current data for pressurized water reactor and boiling water reactor spent nuclear fuel.

In the 1980s, a series of critical experiments referred to as the Haut Taux de Combustion (HTC)
experiments was conducted by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) at the
experimental criticality facility in Valduc, France. The plutonium-to- uranium ratio and the isotopic
compositions of both the uranium and plutonium used in the simulated fuel rods were designed to be
similar to what would be found in a typical pressurized-water reactor fuel assembly that initially had an

In this study, the long-term geochemical behavior of waste package (WP), containing Pu-ceramic, was modeled. The ceramic under consideration contains Ti, U, Pu, Gd and Hf in a pyrochlore structure; the Gd and Hf stabilize the mineral structure, but are also intended to provide criticality control. The specific study objectives were to determine:
1) the extent to which criticality control material, suggested for this WP design, will remain in the WP after corrosion/dissolution of the initial package configuration (such that it can be effective in preventing criticality), and

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

The objective of this calculation is to establish an isotopic database to represent commercial spent nuclear fuel (CSNF) from pressurized water reactors (PWRs) in criticality analyses performed for the proposed Monitored Geologic Repository at Yucca Mountain, Nevada. Confirmation of the conservatism with respect to criticality in the isotopic concentration values represented by this isotopic database is performed as described in Section 3.5.3.1.2 of the Disposal Criticality Analysis Methodology Topical Report (YMP 2000).

The purpose of this study is to provide insights into the neutronic similarities that may exist between a
generic cask containing typical spent nuclear fuel assemblies and commercial reactor critical (CRC) state-
points. Forty CRC state-points from five pressurized-water reactors were selected for the study and the
type of CRC state-points that may be applicable for validation of burnup credit criticality safety
calculations for spent fuel transport/storage/disposal systems are identified. The study employed cross-

The objective of Calculation of Isotopic Bias and Uncertainty for BWR SNF is to quantify the computational bias and uncertainty in the multiplication factor (keff) to be used for Boiling Water Reactor (BWR) spent nuclear fuel (SNF) burn-up credit. The scope of this bias and uncertainty determination covers 38 different radiochemical assay (RCA) spent fuel samples from 14 different fuel assemblies that were irradiated in four different BWRs. The irradiated fuel samples evaluated span an enrichment range of 2.53 weight percent U-235 through 3.95 weight percent U-235.