The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

Spent Fuel Project Office Interim Staff Guidance - 8

Spent Fuel Project Office, Interim Staff Guidance - 8, Revision 1

This research examines the practice of equating the reactivity of spent fuel to that of fresh fuel for the purpose of performing burnup credit criticality safety analyses for PWR spent fuel pool (SFP) storage conditions. The investigation consists of comparing kf estimates based on reactivity "equivalent" fresh fuel enrichment (REFFE) to kl estimates using the actual spent fuel isotopics.

STARBUCS is a new prototypic analysis sequence for performing automated criticality safety analyses of spent fuel systems employing burnup credit. A depletion analysis calculation for each of the burnup-dependent regions of a spent fuel assembly, or other system containing spent fuel, is performed using the ORIGEN-ARP sequence of SCALE. The spent fuel compositions are then used to generate resonance self-shielded cross sections for each region of the problem, which are applied in a three-dimensional criticality safety calculation using the KENO V.a code.

Spent Fuel Project Office, Interim Staff Guidance - 8, Revision 2 - Burnup Credit in the Criticality Safety Analyses of PWR Spent Fuel in Transport
and Storage Casks

As part of a larger program to study mixed-oxide fuel subject to high burnup, some UO2 samples were exposed and analyzed. This report discusses results from the analysis of a UO sample that was burned in a boiling-water reactor (BWR) to approximately 57 GWd/t. The sample

This report has been prepared to qualitatively assess the amount of burnup credit (reactivity margin) provided by ISG-8 compared to that provided by the burnup credit methodology developed and currently applied in France. For the purposes of this study, the methods proposed in the DOE Topical Report have been applied to the ISG-8 framework since this methodology (or one similar to it) is likely to form the basis of initial cask licensing applications employing limited burnup credit in the United States.

The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.