The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

This report describes a novel approach developed at the Oak Ridge National Laboratory
(ORNL) for the estimation of the uncertainty in the prediction of the neutron multiplication factor
for spent nuclear fuel. This technique focuses on burnup credit, where credit is taken in criticality
safety analysis for the reduced reactivity of fuel irradiated in and discharged from a reactor.
Validation methods for burnup credit have attempted to separate the uncertainty associated with

The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

Performance objectives for the geologic repository operations area through permanent closure in 10 CFR 63.111 identify compliance with regulatory dose limits for workers and members of the public as a design objective. The purpose of this design calculation is to determine direct radiation dose consequences for Category 1 and 2 event sequences. It does not include worker dose assessment for recovery operations following Category 1 event sequences.

The objective of this calculation is to provide the uncertainty term for fission product and minor actinides which contributes to the determination of the critical limit for burnup credit calculations. The scope of this calculation covers PWR and BWR spent nuclear fuel. This activity supports the Criticality Department's validation of burnup credit. The intended use of these results is in future Criticality Department calculations and analyses.