This report presents the results of computer code benchmark simulations against spent fuel radiochemical assay
measurements from the Kansai Electric Ltd. Takahama-3 reactor published by the Japan Atomic Energy
Research Institute. Takahama-3 is a pressurized-water reactor that operates with a 17 × 17 fuel-assembly design.
Spent fuel samples were obtained from assemblies operated for 2 and 3 cycles and achieved a maximum burnup
of 47 GWd/MTU. Radiochemical analyses were performed on two rods having an initial enrichment of

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

This report is part of a report series designed to document benchmark-quality radiochemical isotopic
assay data against which computer code accuracy can be quantified to establish the uncertainty and bias
associated with the code predictions. The experimental data included in the report series were acquired
from domestic and international programs and include spent fuel samples that cover a large burnup range.
The measurements analyzed in the current report, for which experimental data is publicly available,

This report presents results from a parametric study of equilibrium fuel cycle costs for a closed fuel cycle with multi-recycling of plutonium in fast reactors (FRs) compared to an open, once-through fuel cycle using PWRs. The study examines the impact on fuel cycle costs from changes in the unit costs of uranium, advanced PUREX reprocessing of discharged uranium dioxide (UO2) fuel and fast-reactor mixed-oxide (FR-MOX) fuel, and FR-MOX fuel fabrication.

Expanding interest in nuclear power and advanced fuel cycles indicate that use of mixed-oxide (MOX) fuel in the current and new U.S. reactor fleet could become an option for utilities in the coming decades. In light of this renewed interest, EPRI has reviewed the substantial knowledge base on MOX fuel irradiation in light water reactors (LWRs). The goal was to evaluate the technical feasibility of MOX fuel use in the U.S. reactor fleet for both existing and advanced LWR designs (Generation III/III+).

Within the context of long-term waste management and sustainable nuclear fuel supply, there continue to be discussions regarding whether the United States should consider recycling of light-water reactor (LWR) spent nuclear fuel (SNF) for the current fleet of U.S. LWRs. This report presents a parametric study of equilibrium fuel cycle costs for an open fuel cycle without plutonium recycling (once-through) and with plutonium recycling (single-recycling using mixed-oxide, or MOX, fuel), assuming an all-pressurized water reactor (PWR) fleet.

The purpose of this study is to provide insights into the neutronic similarities that may exist between a
generic cask containing typical spent nuclear fuel assemblies and commercial reactor critical (CRC) state-
points. Forty CRC state-points from five pressurized-water reactors were selected for the study and the
type of CRC state-points that may be applicable for validation of burnup credit criticality safety
calculations for spent fuel transport/storage/disposal systems are identified. The study employed cross-

Uncertainties in the predicted isotopic concentrations in spent nuclear fuel represent one of the largest
sources of overall uncertainty in criticality calculations that use burnup credit. The methods used to
propagate the uncertainties in the calculated nuclide concentrations to the uncertainty in the predicted
neutron multiplication factor (keff) of the system can have a significant effect on the uncertainty in the
safety margin in criticality calculations and ultimately affect the potential capacity of spent fuel transport

Ever since the 1950s, plutonium, used in fas reactors, has been seen as the key to unlocking the vast energy resource contained in the the world's uranium reserves. However, the reductions in expected nuclear reactor installation rates, combined with discovery of additional uranium, have led to a lengthening in the perceived time interval before fast reactors, the most effective users of plutonium, will make large demands on plutonium supplies. THere are several options concerning its use or storage in the meantime.

This report presents the analyses and results for the potential occurrence of external criticality events which could result from plutonium waste forms emplaced in a geologic repository similar to the one being developed at Yucca Mountain. The analyses evaluate both the MOX spent fuel and the immobilized plutonium waste forms in a repository if the waste package has degraded and if the fissile material has migrated to the invert and out into the far-field.

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.