This report describes a novel approach developed at the Oak Ridge National Laboratory
(ORNL) for the estimation of the uncertainty in the prediction of the neutron multiplication factor
for spent nuclear fuel. This technique focuses on burnup credit, where credit is taken in criticality
safety analysis for the reduced reactivity of fuel irradiated in and discharged from a reactor.
Validation methods for burnup credit have attempted to separate the uncertainty associated with

This report is developed from Technical Work Plan for: Thermodynamic Databases for Chemical Modeling (BSC 2006 [DIRS 177885]). The purpose of this analysis report is to update the thermochemical database data0.ymp.R4 (Output DTN: SN0410T0510404.002). Various data have been added, corrected, or corroborated, partly in response to four Condition Reports (CRs): CR 6489, CR 6731, CR 7542, and CR 7756. The most notable changes are a general revision of phosphate data to achieve consistency with the recommendations from the Committee on Data for Science and Technology (CODATA) (Cox. et al.

The objective of this calculation is to provide the uncertainty term for fission product and minor actinides which contributes to the determination of the critical limit for burnup credit calculations. The scope of this calculation covers PWR and BWR spent nuclear fuel. This activity supports the Criticality Department's validation of burnup credit. The intended use of these results is in future Criticality Department calculations and analyses.