This analysis is prepared by the Mined Geologic Disposal System (MGDS) Waste Package Development (WPD) department to provide a probabilistic evaluation of the potential for criticality of fissile material which has been transported from a geologic repository containing breached waste packages of commercial spent nuclear fuel (SNF). This analysis is part of a continuing investigation of the probability of criticality resulting from the emplacement of spent nuclear fuel in a geologic repository.

This report presents a methodology for validation of the isotopic
contents of spent light water reactor fuel for actinide-only burnup
credit with additional high-quality radiochemistry assay (RCA) data
obtained from the Yankee Rowe pressurized water reactor. The
additional Yankee Rowe RCA data were not included in previous
isotopic validation studies for burnup credit due to the difficulty of
accurately modeling the complex Yankee Rowe fuel assembly design
using the SAS2H one-dimensional sequence of the earlier SCALE

A flat, uniform axial burnup assumption, preferred for its computational simplicity, does not always conservatively estimate the pressurized water reactor spent-fuel-cask multiplication factors. Rather, the reactivity effect of the significantly underburned fuel ends, usually referred to as the "end effect," can be properly treated by explicit modeling of the axial burnup distribution based on limiting axial burnup profiles.

In the 1980s a series of the Haut Taux de Combustion (HTC) critical experiments with fuel pins in a water-moderated lattice was conducted at the Apparatus B experimental facility in Valduc (Commissariat à l'Energie Atomique, France) with the support of the Institut de Radioprotection et de Sûreté Nucléaire and AREVA NC. Four series of experiments were designed to assess profit associated with actinide-only burnup credit in the criticality safety evaluation for fuel handling, pool storage, and spent-fuel cask conditions.

The purpose of this report is to document and validate the external accumulation model that predicts accumulation of fissile materials in the invert, fractures and lithophysae in the rock beneath a degrading waste package containing spent nuclear fuel (SNF) in the monitored geologic repository at Yucca Mountain. (Lithophysae are hollow, bubblelike structures in the rock composed of concentric shells of finely crystalline alkali feldspar, quartz, and other materials (Bates and Jackson 1984 [DIRS 128109], p.

In the 1980s, a series of critical experiments referred to as the Haut Taux de Combustion (HTC)
experiments was conducted by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) at the
experimental criticality facility in Valduc, France. The plutonium-to- uranium ratio and the isotopic
compositions of both the uranium and plutonium used in the simulated fuel rods were designed to be
similar to what would be found in a typical pressurized-water reactor fuel assembly that initially had an

In this study, the long-term geochemical behavior of waste package (WP), containing Pu-ceramic, was modeled. The ceramic under consideration contains Ti, U, Pu, Gd and Hf in a pyrochlore structure; the Gd and Hf stabilize the mineral structure, but are also intended to provide criticality control. The specific study objectives were to determine:
1) the extent to which criticality control material, suggested for this WP design, will remain in the WP after corrosion/dissolution of the initial package configuration (such that it can be effective in preventing criticality), and

The Disposal Criticality Analysis Methodology Topical Report (Reference 1) states that the accuracy of the criticality analysis methodology (MCNP Monte Carlo code and cross-section data) designated to assess the potential for criticality of various configurations in the Yucca Mountain proposed repository is established by evaluating appropriately selected benchmark critical experiments.

This study is prepared by the Mined Geologic Disposal System (MODS) Waste Package Development Department (WPDD) to provide input to a separate evaluation on the probablility of criticality in the far- field environment. These calculations are performed in sufficient detail to provide conservatively bounding configurations to support separate probabilistic analyses.

This report presents the analyses and results for the potential occurrence of external criticality events which could result from plutonium waste forms emplaced in a geologic repository similar to the one being developed at Yucca Mountain. The analyses evaluate both the MOX spent fuel and the immobilized plutonium waste forms in a repository if the waste package has degraded and if the fissile material has migrated to the invert and out into the far-field.