The objective of these calculations is to perform intact and degraded mode criticality evaluations of the Department of Energy's (DOE) Three Mile Island- Unit 2 (TMI-2) spent nuclear fuel (SNF) in canisters. This analysis evaluates codisposal in a 5-Defense High-Level Waste (5-DHLW/DOE SNF) Long Waste Package (Civilian Radioactive Waste Management System Management and Operating Contractor [CRWMS M&O] 2000b, Attachment V), which is to be placed in a potential monitored geologic repository (MGR).

This report presents a methodology for validation of the isotopic
contents of spent light water reactor fuel for actinide-only burnup
credit with additional high-quality radiochemistry assay (RCA) data
obtained from the Yankee Rowe pressurized water reactor. The
additional Yankee Rowe RCA data were not included in previous
isotopic validation studies for burnup credit due to the difficulty of
accurately modeling the complex Yankee Rowe fuel assembly design
using the SAS2H one-dimensional sequence of the earlier SCALE

A flat, uniform axial burnup assumption, preferred for its computational simplicity, does not always conservatively estimate the pressurized water reactor spent-fuel-cask multiplication factors. Rather, the reactivity effect of the significantly underburned fuel ends, usually referred to as the "end effect," can be properly treated by explicit modeling of the axial burnup distribution based on limiting axial burnup profiles.

Criticality safety analysis devoted to spent-fuel storage and transportation has to be conservative in order to be sure no accident will ever happen. In the spent-fuel storage field, the assumption of freshness has been used to achieve the conservative aspect of criticality safety procedures. Nevertheless, after being irradiated in a reactor core, the fuel elements have obviously lost part of their original reactivity. The concept of taking into account this reactivity loss in criticality safety analysis is known as burnup credit.

In the 1980s a series of the Haut Taux de Combustion (HTC) critical experiments with fuel pins in a water-moderated lattice was conducted at the Apparatus B experimental facility in Valduc (Commissariat à l'Energie Atomique, France) with the support of the Institut de Radioprotection et de Sûreté Nucléaire and AREVA NC. Four series of experiments were designed to assess profit associated with actinide-only burnup credit in the criticality safety evaluation for fuel handling, pool storage, and spent-fuel cask conditions.

In the 1980s, a series of critical experiments referred to as the Haut Taux de Combustion (HTC)
experiments was conducted by the Institut de Radioprotection et de Sûreté Nucléaire (IRSN) at the
experimental criticality facility in Valduc, France. The plutonium-to- uranium ratio and the isotopic
compositions of both the uranium and plutonium used in the simulated fuel rods were designed to be
similar to what would be found in a typical pressurized-water reactor fuel assembly that initially had an