The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

As nuclear power plants began to run out of storage capacity in spent nuclear fuel (SNF) storage pools, many nuclear operating companies added higher density pool storage racks to increase pool capacity. Most nuclear power plant storage pools have been re-racked one or more times. As many spent fuel storage pools were re-racked to the maximum extent possible, nuclear operating companies began to employ interim dry storage technologies to store SNF in certified casks and canister-based systems outside of the storage pool in independent spent fuel storage installations (ISFSIs).

Independent spent fuel storage installations (ISFSIs) are currently licensed for 20 years. However, delays in developing permanent spent fuel disposal capability require continued ISFSI storage beyond the 20-year term. This report provides a technical basis for demonstrating the feasibility of extended spent fuel storage in ISFSIs.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

Isotopic characterization of spent fuel via depletion and decay calculations is necessary for
determination of source terms for subsequent system analyses involving heat transfer, radiation
shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality
safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and
decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in

The work reported here is an investigation of the sensitivity of component temperatures in a specific storage system, including fuel cladding temperatures, in response to modeling assumptions that differ from design-basis, including age-related changes that could degrade the thermal behavior of the system. Preliminary evaluations of representative horizontal and vertical storage systems at design basis conditions provides general insight into the expected behavior of storage systems over extended periods of time.

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