The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

This report presents results from a parametric study of equilibrium fuel cycle costs for a closed fuel cycle with multi-recycling of plutonium in fast reactors (FRs) compared to an open, once-through fuel cycle using PWRs. The study examines the impact on fuel cycle costs from changes in the unit costs of uranium, advanced PUREX reprocessing of discharged uranium dioxide (UO2) fuel and fast-reactor mixed-oxide (FR-MOX) fuel, and FR-MOX fuel fabrication.

Expanding interest in nuclear power and advanced fuel cycles indicate that use of mixed-oxide (MOX) fuel in the current and new U.S. reactor fleet could become an option for utilities in the coming decades. In light of this renewed interest, EPRI has reviewed the substantial knowledge base on MOX fuel irradiation in light water reactors (LWRs). The goal was to evaluate the technical feasibility of MOX fuel use in the U.S. reactor fleet for both existing and advanced LWR designs (Generation III/III+).

Within the context of long-term waste management and sustainable nuclear fuel supply, there continue to be discussions regarding whether the United States should consider recycling of light-water reactor (LWR) spent nuclear fuel (SNF) for the current fleet of U.S. LWRs. This report presents a parametric study of equilibrium fuel cycle costs for an open fuel cycle without plutonium recycling (once-through) and with plutonium recycling (single-recycling using mixed-oxide, or MOX, fuel), assuming an all-pressurized water reactor (PWR) fleet.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
(AFR) criticality safety analyses be validated against experimental measurements. If credit for the
negative reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark AFR criticality analysis methods using selected critical
configurations from commercial pressurized-water reactors (PWR).

STARBUCS is a new prototypic analysis sequence for performing automated criticality safety analyses of spent fuel systems employing burnup credit. A depletion analysis calculation for each of the burnup-dependent regions of a spent fuel assembly, or other system containing spent fuel, is performed using the ORIGEN-ARP sequence of SCALE. The spent fuel compositions are then used to generate resonance self-shielded cross sections for each region of the problem, which are applied in a three-dimensional criticality safety calculation using the KENO V.a code.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit for the negative
reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark away-from-reactor criticality analysis methods using critical
configurations from commercial pressurized-water reactors.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

Isotopic characterization of spent fuel via depletion and decay calculations is necessary for
determination of source terms for subsequent system analyses involving heat transfer, radiation
shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality
safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and
decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in

Five commercial reactor criticals (CRCs) for the LaSalle Unit 1 boiling-water reactor
have been analyzed using KENO V.a, the Monte Carlo criticality code of the SCALE 4 code
system. The irradiated fuel assembly isotopics for the criticality analyses were provided by the
Waste Package Design team at the Yucca Mountain Project in the United States, who performed
the depletion calculations using the SAS2H sequence of SCALE 4. The reactor critical
measurements involved two beginning-of-cycle and three middle-of-cycle configurations. The

The requirements of ANSI/ANS-8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original "fresh" composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

This report is part of a report series designed to document benchmark-quality radiochemical assay data
against which computer code predictions of isotopic composition for spent nuclear fuel can be validated
to establish the uncertainty and bias associated with the code predictions. The experimental data analyzed
in the present report were acquired from two international programs: (1) ARIANE and (2) REBUS, both
coordinated by Belgonucleaire. All measurements include extensive actinide and fission product data of

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original $fresh# composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.

Ever since the 1950s, plutonium, used in fas reactors, has been seen as the key to unlocking the vast energy resource contained in the the world's uranium reserves. However, the reductions in expected nuclear reactor installation rates, combined with discovery of additional uranium, have led to a lengthening in the perceived time interval before fast reactors, the most effective users of plutonium, will make large demands on plutonium supplies. THere are several options concerning its use or storage in the meantime.

This report presents the analyses and results for the potential occurrence of external criticality events which could result from plutonium waste forms emplaced in a geologic repository similar to the one being developed at Yucca Mountain. The analyses evaluate both the MOX spent fuel and the immobilized plutonium waste forms in a repository if the waste package has degraded and if the fissile material has migrated to the invert and out into the far-field.

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.