The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

Taking credit for the reduced reactivity of spent nuclear fuel in criticality analyses is referred to
as burnup credit. Criticality safety evaluations employing burnup credit require validation of the
depletion and criticality calculation methods and computer codes with available measurement
data. To address the issues of burnup credit criticality validation, the U.S. Nuclear Regulatory
Commission initiated a project with Oak Ridge National Laboratory to (1) develop and establish

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
(AFR) criticality safety analyses be validated against experimental measurements. If credit for the
negative reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark AFR criticality analysis methods using selected critical
configurations from commercial pressurized-water reactors (PWR).

STARBUCS is a new prototypic analysis sequence for performing automated criticality safety analyses of spent fuel systems employing burnup credit. A depletion analysis calculation for each of the burnup-dependent regions of a spent fuel assembly, or other system containing spent fuel, is performed using the ORIGEN-ARP sequence of SCALE. The spent fuel compositions are then used to generate resonance self-shielded cross sections for each region of the problem, which are applied in a three-dimensional criticality safety calculation using the KENO V.a code.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit for the negative
reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark away-from-reactor criticality analysis methods using critical
configurations from commercial pressurized-water reactors.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

The purpose of this study is to provide insights into the neutronic similarities that may exist between a
generic cask containing typical spent nuclear fuel assemblies and commercial reactor critical (CRC) state-
points. Forty CRC state-points from five pressurized-water reactors were selected for the study and the
type of CRC state-points that may be applicable for validation of burnup credit criticality safety
calculations for spent fuel transport/storage/disposal systems are identified. The study employed cross-

Isotopic characterization of spent fuel via depletion and decay calculations is necessary for
determination of source terms for subsequent system analyses involving heat transfer, radiation
shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality
safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and
decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in

Five commercial reactor criticals (CRCs) for the LaSalle Unit 1 boiling-water reactor
have been analyzed using KENO V.a, the Monte Carlo criticality code of the SCALE 4 code
system. The irradiated fuel assembly isotopics for the criticality analyses were provided by the
Waste Package Design team at the Yucca Mountain Project in the United States, who performed
the depletion calculations using the SAS2H sequence of SCALE 4. The reactor critical
measurements involved two beginning-of-cycle and three middle-of-cycle configurations. The

The requirements of ANSI/ANS-8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original "fresh" composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

Spent fuel transportation and storage cask designs based on a burnup credit approach must
consider issues that are not relevant in casks designed under a fresh-fuel loading assumption. For
example, the spent fuel composition must be adequately characterized and the criticality analysis
model can be complicated by the need to consider axial burnup variations. Parametric analyses are
needed to characterize the importance of fuel assembly and fuel cycle parameters on spent fuel

This report is part of a report series designed to document benchmark-quality radiochemical assay data
against which computer code predictions of isotopic composition for spent nuclear fuel can be validated
to establish the uncertainty and bias associated with the code predictions. The experimental data analyzed
in the present report were acquired from two international programs: (1) ARIANE and (2) REBUS, both
coordinated by Belgonucleaire. All measurements include extensive actinide and fission product data of

Taking credit for the reduced reactivity of spent nuclear fuel (SNF) in criticality analyses is referred to as burnup credit (BUC). Criticality safety evaluations require validation of the computational methods with critical experiments that are as similar as possible to the safety analysis models, and for which the keff values are known. This poses a challenge for validation of BUC criticality analyses, as critical experiments with actinide and fission product (FP)

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original $fresh# composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.