The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

This report proposes and documents a computational benchmark for the estimation of the
additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor
actinides in a burnup-credit storage/transport environment, relative to SNF compositions
containing only the major actinides. The benchmark problem/configuration is a generic burnupcredit
cask designed to hold 68 boiling water reactor (BWR) spent nuclear fuel assemblies. The
purpose of this computational benchmark is to provide a reference configuration for the

This report has been prepared to support technical discussion of and planning for future
research supporting implementation of burnup credit for boiling-water reactor (BWR) spent fuel
storage in spent fuel pools and storage and transport cask applications. The review and
discussion in this report are based on knowledge and experience gained from work performed
in the United States and other countries, including experience with burnup credit for
pressurized-water reactor (PWR) spent fuel. Relevant physics and analysis phenomena are

This report presents a best-estimate probabilistic risk assessment (PRA) to quantify the frequency of criticality accidents during railroad transportation of spent nuclear fuel casks. The assessment is of sufficient detail to enable full scrutiny of the model logic and the basis for each quantitative parameter contributing to criticality accident scenario frequencies. The report takes into account the results of a 2007 peer review of the initial version of this probabilistic risk assessment, which was published as EPRI Technical Report 1013449 in December 2006.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
(AFR) criticality safety analyses be validated against experimental measurements. If credit for the
negative reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark AFR criticality analysis methods using selected critical
configurations from commercial pressurized-water reactors (PWR).

Utilization of burnup credit in criticality safety analysis for long-term disposal of spent
nuclear fuel allows improved design efficiency and reduced cost due to the large mass of fissile
material that will be present in the repository. Burnup-credit calculations are based on depletion
calculations that provide a conservative estimate of spent fuel contents (in terms of criticality
potential), followed by criticality calculations to assess the value of the effective neutron

STARBUCS is a new prototypic analysis sequence for performing automated criticality safety analyses of spent fuel systems employing burnup credit. A depletion analysis calculation for each of the burnup-dependent regions of a spent fuel assembly, or other system containing spent fuel, is performed using the ORIGEN-ARP sequence of SCALE. The spent fuel compositions are then used to generate resonance self-shielded cross sections for each region of the problem, which are applied in a three-dimensional criticality safety calculation using the KENO V.a code.

This report investigates trends in the radiological decay properties and changes in relative nuclide importance associated with increasing enrichments and burnup for spent LWR fuel as they affect the areas of criticality safety, thermal analysis (decay heat), and shielding analysis of spent fuel transport and storage casks. To facilitate identifying the changes in the spent fuel compositions that most directly impact these application areas, the dominant nuclides in each area have been identified and ranked by importance.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit for the negative
reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark away-from-reactor criticality analysis methods using critical
configurations from commercial pressurized-water reactors.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

Isotopic characterization of spent fuel via depletion and decay calculations is necessary for
determination of source terms for subsequent system analyses involving heat transfer, radiation
shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality
safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and
decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in

Five commercial reactor criticals (CRCs) for the LaSalle Unit 1 boiling-water reactor
have been analyzed using KENO V.a, the Monte Carlo criticality code of the SCALE 4 code
system. The irradiated fuel assembly isotopics for the criticality analyses were provided by the
Waste Package Design team at the Yucca Mountain Project in the United States, who performed
the depletion calculations using the SAS2H sequence of SCALE 4. The reactor critical
measurements involved two beginning-of-cycle and three middle-of-cycle configurations. The

The requirements of ANSI/ANS-8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original "fresh" composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

This report is part of a report series designed to document benchmark-quality radiochemical assay data
against which computer code predictions of isotopic composition for spent nuclear fuel can be validated
to establish the uncertainty and bias associated with the code predictions. The experimental data analyzed
in the present report were acquired from two international programs: (1) ARIANE and (2) REBUS, both
coordinated by Belgonucleaire. All measurements include extensive actinide and fission product data of

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit is to be taken for
the reduced reactivity of burned or spent fuel relative to its original $fresh# composition, it is
necessary to benchmark computational methods used in determining such reactivity worth against
spent fuel reactivity measurements. This report summarizes a portion of the ongoing effort to

The validity of the computation of pressurized-water-reactor (PWR) spent fuel isotopic
composition by the SCALE system depletion analysis was assessed using data presented in the report.
Radiochemical measurements and SCALE/SAS2H computations of depleted fuel isotopics were
compared with 19 benchmark-problem samples from Calvert Cliffs Unit 1, H. B. Robinson Unit 2,
and Obrigheim PWRs. Even though not exhaustive in scope, the validation included comparison of
predicted and measured concentrations for 14 actinides and 37 fission and activation products.

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.