The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

The U.S. Nuclear Regulatory Commission (NRC) is evaluating the safety and security of spent nuclear fuel (SNF) stored in dry casks for extended time periods before transportation to a location where the SNF is further processed or permanently disposed.

Isotopic characterization of spent fuel via depletion and decay calculations is necessary for
determination of source terms for subsequent system analyses involving heat transfer, radiation
shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality
safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and
decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in

Several hundred distinct types of DOE-owned spent nuclear fuel (DSNF) may potentially be disposed in the Yucca Mountain repository. These fuel types represent many more types than can be viably individually examined for their effect on the Total System Performance Assessment for the License Application (TSPA-LA). Additionally, for most of these fuel types, there is no known direct experimental test data for the degradation and dissolution of the waste form in repository groundwaters.