This “Technical Evaluation Report on the Content of the U.S. Department of Energy’s Yucca Mountain License Application; Postclosure Volume: Repository Safety After Permanent Closure” (TER Postclosure Volume) presents information on the NRC staff’s review of DOE’s Safety Analysis Report (SAR), provided on June 3, 2008, as updated by DOE on February 19, 2009. The NRC staff also reviewed information DOE provided in response to NRC staff’s requests for additional information and other information that DOE provided related to the SAR.

This analysis provides information necessary for total system performance assessment (TSPA) for the license application (LA) to include the excess U.S. Department of Energy (DOE) plutonium in the form of mixed oxide (MOX) spent nuclear fuel and lanthanide borosilicate (LaBS) glass. This information includes the additional radionuclide inventory due to MOX spent nuclear fuel and LaBS glass and the analysis that shows that the TSPA models for commercial spent nuclear fuel (CSNF) and high-level waste (HLW) degradation are appropriate for MOX spent nuclear fuel and LaBS glass, respectively.

Taking credit for the reduced reactivity of spent nuclear fuel in criticality analyses is referred to
as burnup credit. Criticality safety evaluations employing burnup credit require validation of the
depletion and criticality calculation methods and computer codes with available measurement
data. To address the issues of burnup credit criticality validation, the U.S. Nuclear Regulatory
Commission initiated a project with Oak Ridge National Laboratory to (1) develop and establish

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of the mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.

The purpose of this analysis is to provide an initial radionuclide inventory (in grams per waste package) and associated uncertainty distributions for use in the Total System Performance Assessment for the License Application (TSPA-LA) in support of the license application for the repository at Yucca Mountain, Nevada. This document is intended for use in postclosure analysis only.

The means to prevent and control criticality must be addressed as part of the Preclosure Safety Analysis (PCSA) required for compliance with 10 CFR Part 63 [DIRS 180319], where the preclosure period covers the time prior to permanent closure activities. This technical report presents the nuclear criticality safety evaluation that documents the achievement of this objective.

From 1998 to 2004, a series of critical experiments referred to as the fission product (FP) experimental program was performed at the Commissariat à l'Energie Atomique Valduc research facility. The experiments were designed by Institut de Radioprotection et de Sûreté Nucléaire (IRSN) and funded by AREVA NC and IRSN within the French program supporting development of a technical basis for burnup credit validation.

This report proposes and documents a computational benchmark for the estimation of the
additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor
actinides in a burnup-credit storage/transport environment, relative to SNF compositions
containing only the major actinides. The benchmark problem/configuration is a generic burnupcredit
cask designed to hold 68 boiling water reactor (BWR) spent nuclear fuel assemblies. The
purpose of this computational benchmark is to provide a reference configuration for the

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

Past efforts by the Department of Energy (DOE), the Electric Power Research Institute (EPRI), the Nuclear Regulatory Commission (NRC), and others have provided sufficient technical information to enable the NRC to issue regulatory guidance for implementation of pressurized-water reactor (PWR) burnup credit; however, consideration of only the reactivity change due to the major actinides is recommended in the guidance.

The purpose of this report is to document calculations of the number of waste packages that could be damaged in a potential future igneous event intersecting a repository at YuccaMountain. The analyses include disruption from an igneous intrusion and from an igneous eruption. The analyses also support the evaluation of the potential consequences from a future event as part of the total system performance assessment (TSPA) for the license application for the Yucca Mountain Project.

The purpose of this calculation is to perform a parametric study to determine the effects of fission product leaching, assembly collapse, and iron oxide loss on the reactivity of a waste package containing mixed oxide spent nuclear fuel. Previous calculations (CRWMS M&O 1998a) have shown that the criticality control features of the waste package are adequate to prevent criticality of a flooded WP for all the enrichment/burnup pairs expected for the MOX SNF.

This report was developed in accordance with the requirements in Technical Work Plan for Postclosure Waste Form Modeling (BSC 2005 [DIRS 173246]). The purpose of the in-package chemistry model is to predict the bulk chemistry inside of a breached waste package and to provide simplified expressions of that chemistry as a function of time after breach to Total Systems Performance Assessment for the License Application (TSPA-LA).

Optimization of energy resources suggests increased fuel residence in reactor cores and hence improved
fission product evaluations are required. For thermal reactors the fission product cross sections in the JEF2.2 and
JEFF3.1 libraries plus new evaluations from WPEC23 are assessed through modelling the CERES experiment in
the DIMPLE reactor. The analysis uses the lattice code WIMS10. Cross sections for 12 nuclides are assessed. The
thermal cross section and low energy resonance data for 147,152Sm and 155Gd are accurate to within 4%. Similar data

U.S. Nuclear Regulatory Commission Interim Staff Guidance 8 (ISG-8) for burnup credit covers actinides only, a position based primarily on the lack of definitive critical experiments and adequate radiochemical assay data that can be used to quantify the uncertainty associated with fission product credit.

The objective of Calculation of Isotopic Bias and Uncertainty for BWR SNF is to quantify the computational bias and uncertainty in the multiplication factor (keff) to be used for Boiling Water Reactor (BWR) spent nuclear fuel (SNF) burn-up credit. The scope of this bias and uncertainty determination covers 38 different radiochemical assay (RCA) spent fuel samples from 14 different fuel assemblies that were irradiated in four different BWRs. The irradiated fuel samples evaluated span an enrichment range of 2.53 weight percent U-235 through 3.95 weight percent U-235.

The objective of the Limerick Unit 1 Radiochemical Assay Comparisons to SAS2H Calculations is to determine the accuracy of the SAS2H control module of the baselined modular code system SCALE, Version 4.4A (STN: 10129-4.4A-00), in predicting the isotopic concentrations of spent fuel, and to quantify the overall effect that the differences between the calculated and measured isotopic concentrations have on the system reactivity. The scope of this calculation covers eight different spent fuel samples from a fuel assembly that was irradiated in the Limerick Unit 1 boiling water reactor (BWR).

The purpose of this analysis report is to develop the summary cladding degradation abstraction that will be used in the Total System Performance Assessment for the License Application (TSPA-LA). Most civilian commercial nuclear fuel is encased in Zircaloy cladding. The analysis addressed in this report is intended to describe the postulated condition of commercial Zircaloy-clad fuel as a function of postclosure time after it is placed in the repository.