Taking credit for the reduced reactivity of spent nuclear fuel in criticality analyses is referred to
as burnup credit. Criticality safety evaluations employing burnup credit require validation of the
depletion and criticality calculation methods and computer codes with available measurement
data. To address the issues of burnup credit criticality validation, the U.S. Nuclear Regulatory
Commission initiated a project with Oak Ridge National Laboratory to (1) develop and establish

The purpose of the material degradation and release (MDR) model is to predict the fate of the waste package materials, specifically the retention or mobilization of the radionuclides and the neutron-absorbing material as a function of time after the breach of a waste package during the 10,000 years after repository closure. The output of this model is used directly to assess the potential for a criticality event inside the waste package due to the retention of the radionuclides combined with a loss of the neutron-absorbing material.

From 1998 to 2004, a series of critical experiments referred to as the fission product (FP) experimental program was performed at the Commissariat à l'Energie Atomique Valduc research facility. The experiments were designed by Institut de Radioprotection et de Sûreté Nucléaire (IRSN) and funded by AREVA NC and IRSN within the French program supporting development of a technical basis for burnup credit validation.

This report proposes and documents a computational benchmark for the estimation of the
additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor
actinides in a burnup-credit storage/transport environment, relative to SNF compositions
containing only the major actinides. The benchmark problem/configuration is a generic burnupcredit
cask designed to hold 68 boiling water reactor (BWR) spent nuclear fuel assemblies. The
purpose of this computational benchmark is to provide a reference configuration for the

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

The purpose and scope of this model report is to document models for general and localized corrosion of the waste package outer barrier (WPOB) to be used in evaluating long-term waste package performance in the total system performance assessment (TSPA). The waste package design for the license application is a double-wall waste package placed underneath a protective drip shield (SNL 2007 [DIRS 179394]; SNL 2007 [DIRS 179354]). The WPOB will be constructed of Alloy 22 (UNS N06022) (SNL 2007 [DIRS 179567], Section 4.1.1.6), a highly corrosion-resistant nickel-based alloy.

Past efforts by the Department of Energy (DOE), the Electric Power Research Institute (EPRI), the Nuclear Regulatory Commission (NRC), and others have provided sufficient technical information to enable the NRC to issue regulatory guidance for implementation of pressurized-water reactor (PWR) burnup credit; however, consideration of only the reactivity change due to the major actinides is recommended in the guidance.

The purpose of this calculation is to perform a parametric study to determine the effects of fission product leaching, assembly collapse, and iron oxide loss on the reactivity of a waste package containing mixed oxide spent nuclear fuel. Previous calculations (CRWMS M&O 1998a) have shown that the criticality control features of the waste package are adequate to prevent criticality of a flooded WP for all the enrichment/burnup pairs expected for the MOX SNF.

Stress corrosion cracking (SCC) is one of the most common corrosion-related causes for premature breach of metal structural components. SCC is the initiation and propagation of cracks in structural components due to three factors that must be present simultaneously (Jones 1992 [DIRS 169906], Section 8.1): metallurgical susceptibility, critical environment, and sustained tensile stresses.

This report was developed in accordance with the requirements in Technical Work Plan for Postclosure Waste Form Modeling (BSC 2005 [DIRS 173246]). The purpose of the in-package chemistry model is to predict the bulk chemistry inside of a breached waste package and to provide simplified expressions of that chemistry as a function of time after breach to Total Systems Performance Assessment for the License Application (TSPA-LA).

Optimization of energy resources suggests increased fuel residence in reactor cores and hence improved
fission product evaluations are required. For thermal reactors the fission product cross sections in the JEF2.2 and
JEFF3.1 libraries plus new evaluations from WPEC23 are assessed through modelling the CERES experiment in
the DIMPLE reactor. The analysis uses the lattice code WIMS10. Cross sections for 12 nuclides are assessed. The
thermal cross section and low energy resonance data for 147,152Sm and 155Gd are accurate to within 4%. Similar data

U.S. Nuclear Regulatory Commission Interim Staff Guidance 8 (ISG-8) for burnup credit covers actinides only, a position based primarily on the lack of definitive critical experiments and adequate radiochemical assay data that can be used to quantify the uncertainty associated with fission product credit.

The purpose of this report is to evaluate the potential for penetration of the Alloy 22 (UNS N06022) waste package outer barrier by localized corrosion due to the deliquescence of soluble constituents in dust present on waste package surfaces. The results support a recommendation to exclude deliquescence-induced localized corrosion (pitting or crevice corrosion) of the outer barrier from the total system performance assessment for the license application (TSPA-LA).

The repository design includes a drip shield (BSC 2004 [DIRS 168489]) that provides protection for the waste package both as a barrier to seepage water contact and a physical barrier to potential rockfall.
The purpose of the process-level models developed in this report is to model dry oxidation, general corrosion, and localized corrosion of the drip shield plate material, which is made of Ti Grade 7. This document is prepared ·according to Technical Work Plan For: Regulatory Integration Modeling and Analysis of the Waste Form and Waste Package (BSC 2004 [DIRS 171583]).

The purpose of this analysis is to evaluate the types of defects or imperfections that could occur in a waste package or a drip shield and potentially lead to its early failure, and to estimate a probability of undetected occurrence for each type. An early failure is defined as the through-wall penetration of a waste package or drip shield due to manufacturing or handling-induced defects, at a time earlier than would be predicted by mechanistic degradation models for a defect-free waste package or drip shield.

Hydrogen-induced cracking is characterized by the decreased ductility and fracture toughness of a material due to the absorption of atomic hydrogen in the metal crystal lattice. Corrosion is the source of hydrogen generation. For the current design of the engineered barrier without backfill, hydrogen-induced cracking may be a concern because the titanium drip shield can be galvanically coupled to rock bolts (or wire mesh), which may fall onto the drip shield, thereby creating conditions for hydrogen production by electrochemical reaction.

Taking credit for the reduced reactivity of spent nuclear fuel (SNF) in criticality analyses is referred to as burnup credit (BUC). Criticality safety evaluations require validation of the computational methods with critical experiments that are as similar as possible to the safety analysis models, and for which the keff values are known. This poses a challenge for validation of BUC criticality analyses, as critical experiments with actinide and fission product (FP)

The purpose of this report is to evaluate the potential for penetration of the Alloy 22 (UNS N06022) waste package outer barrier by localized corrosion due to the deliquescence of soluble constituents in dust present on waste package surfaces. The results support a recommendation to exclude deliquescence-induced localized corrosion (pitting or crevice corrosion) of the outer barrier from the total system performance assessment for the license application (TSPA-LA).

This report proposes and documents a computational benchmark problem for the estimation of the additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor actinides in a burnupcredit storage/transport environment, relative to SNF compositions containing only the major actinides. The benchmark problemlconfiguration is a generic burnup credit cask designed to hold 32 pressurized water reactor (PWR) assemblies.

Analytical methods, described in this report, are used to
systematically determine experimental fuel sub-batch
reactivities as a function of burnup. Fuel sub-batch reactivities
are inferred using more than 600 in-core pressurized water
reactor (PWR) flux maps taken during 44 cycles of operation
at the Catawba and McGuire nuclear power plants. The
analytical methods systematically search for fuel sub-batch
reactivities that minimize differences between measured and
computed reaction rates, using Studsvik Scandpower’s