Taking credit for the reduced reactivity of spent nuclear fuel in criticality analyses is referred to
as burnup credit. Criticality safety evaluations employing burnup credit require validation of the
depletion and criticality calculation methods and computer codes with available measurement
data. To address the issues of burnup credit criticality validation, the U.S. Nuclear Regulatory
Commission initiated a project with Oak Ridge National Laboratory to (1) develop and establish

The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

The Monitored Geologic Repository Waste Package Operations of the Civilian Radioactive Waste Management System Management & Operating Contractor (CRWMS M&O) performed calculations to provide input for disposal of spent nuclear fuel (SNF) from the Navy (Refs. 1 and , 2). The Navy SNF has been considered for disposal at the potential Yucca Mountain site. For some waste packages, the containment may breach (Ref. 3), allowing the influx of water. Water in the waste package may moderate neutrons, increasing the likelihood of a criticality event within the waste package.

From 1998 to 2004, a series of critical experiments referred to as the fission product (FP) experimental program was performed at the Commissariat à l'Energie Atomique Valduc research facility. The experiments were designed by Institut de Radioprotection et de Sûreté Nucléaire (IRSN) and funded by AREVA NC and IRSN within the French program supporting development of a technical basis for burnup credit validation.

This report proposes and documents a computational benchmark for the estimation of the
additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor
actinides in a burnup-credit storage/transport environment, relative to SNF compositions
containing only the major actinides. The benchmark problem/configuration is a generic burnupcredit
cask designed to hold 68 boiling water reactor (BWR) spent nuclear fuel assemblies. The
purpose of this computational benchmark is to provide a reference configuration for the

Pressurized water reactor (PWR) burnup credit validation is
demonstrated using the benchmarks for quantifying fuel reactivity
decrements, published as Benchmarks for Quantifying Fuel Reactivity
Depletion Uncertainty, Electric Power Research Institute (EPRI)
report 1022909. This demonstration uses the depletion module
TRITON (Transport Rigor Implemented with Time-Dependent
Operation for Neutronic Depletion) available in the SCALE 6.1
(Standardized Computer Analyses for Licensing Evaluations) code

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

A methodology for performing and applying nuclear criticality safety calculations, for PWR spent nuclear fuel (SNF) packages with actinide-only burnup credit, is described. The changes in the U-234, U-235, U-236, U-238, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, and Am-241 concentration with burnup are used in burnup credit criticality analyses. No credit for fission product neutron absorbers is taken. The methodology consists of five major steps. (1) Validate a computer code system to calculate isotopic concentrations of SNF created during burnup in the reactor core and subsequent decay.

Past efforts by the Department of Energy (DOE), the Electric Power Research Institute (EPRI), the Nuclear Regulatory Commission (NRC), and others have provided sufficient technical information to enable the NRC to issue regulatory guidance for implementation of pressurized-water reactor (PWR) burnup credit; however, consideration of only the reactivity change due to the major actinides is recommended in the guidance.

The Monitored Geologic Repository (MGR) Waste Package Operations (WPO) of the Civilian Radioactive Waste Management System Management & Operating Contractor (CRWMS M&O) performed calculations to provide input for disposal of spent nuclear fuel (SNF) from the Emico Fermi Atomic Power Plant (Ref. 1). The Fermi fuel has been considered for disposal at the potential Yucca Mountain site.

The purpose of this calculation is to perform a parametric study to determine the effects of fission product leaching, assembly collapse, and iron oxide loss on the reactivity of a waste package containing mixed oxide spent nuclear fuel. Previous calculations (CRWMS M&O 1998a) have shown that the criticality control features of the waste package are adequate to prevent criticality of a flooded WP for all the enrichment/burnup pairs expected for the MOX SNF.

Optimization of energy resources suggests increased fuel residence in reactor cores and hence improved
fission product evaluations are required. For thermal reactors the fission product cross sections in the JEF2.2 and
JEFF3.1 libraries plus new evaluations from WPEC23 are assessed through modelling the CERES experiment in
the DIMPLE reactor. The analysis uses the lattice code WIMS10. Cross sections for 12 nuclides are assessed. The
thermal cross section and low energy resonance data for 147,152Sm and 155Gd are accurate to within 4%. Similar data

U.S. Nuclear Regulatory Commission Interim Staff Guidance 8 (ISG-8) for burnup credit covers actinides only, a position based primarily on the lack of definitive critical experiments and adequate radiochemical assay data that can be used to quantify the uncertainty associated with fission product credit.

Fuel from the Fast Flux Test Facility ' (FFTF) has been considered for disposal at the proposed

The Monitored Geologic Repository Waste Package Operations of the Civilian Radioactive Waste Management System Management & Operating Contractor (CRWMS M&O) performed calculations to provide input for disposal of spent nuclear fuel (SNF) from the Training, Research, Isotopes, General Atomics (TRIGA) reactor (Ref. 1). The TRIGA SNF has been considered for disposal at the potential Yucca Mountain site.

The Monitored Geologic Repository (MGR) Waste Package Department of the Civilian Radioactive Waste Management System Management & Operating contractor (CRWMS M&O) performed calculations to provide input for disposal of spent nuclear fuel (SNF) from the Shippingport Light Water Breeder Reactor (LWBR) (Ref. 1). The Shippingport LWBR SNF has been considered for disposal at the potential Yucca Mountain site.

Taking credit for the reduced reactivity of spent nuclear fuel (SNF) in criticality analyses is referred to as burnup credit (BUC). Criticality safety evaluations require validation of the computational methods with critical experiments that are as similar as possible to the safety analysis models, and for which the keff values are known. This poses a challenge for validation of BUC criticality analyses, as critical experiments with actinide and fission product (FP)

This report presents a two-phased approach to develop and analyze a “thermal envelope” to represent the postclosure response of the repository to the anticipated range of repository design thermal loadings. In Phase 1 an estimated limiting waste stream (ELWS) is identified and analyzed to determine the extremes of average and local thermal loading conditions. The coldest thermal loading condition is represented by an emplacement drift loaded exclusively with high-level radioactive waste (HLW) and/or defense spent nuclear fuel (DSNF).

This report is developed from Technical Work Plan for: Thermodynamic Databases for Chemical Modeling (BSC 2006 [DIRS 177885]). The purpose of this analysis report is to update the thermochemical database data0.ymp.R4 (Output DTN: SN0410T0510404.002). Various data have been added, corrected, or corroborated, partly in response to four Condition Reports (CRs): CR 6489, CR 6731, CR 7542, and CR 7756. The most notable changes are a general revision of phosphate data to achieve consistency with the recommendations from the Committee on Data for Science and Technology (CODATA) (Cox. et al.

This report proposes and documents a computational benchmark problem for the estimation of the additional reactivity margin available in spent nuclear fuel (SNF) from fission products and minor actinides in a burnupcredit storage/transport environment, relative to SNF compositions containing only the major actinides. The benchmark problemlconfiguration is a generic burnup credit cask designed to hold 32 pressurized water reactor (PWR) assemblies.

This report documents the development and validation of the in-drift precipitates/salts (IDPS) process model. The IDPS process model is a geochemical model designed to predict the postclosure effects of evaporation and deliquescence on the chemical composition of water within the Engineered Barrier System (EBS) in support of the total system performance assessment (TSPA). Application of the model in support of TSPA is documented in Engineered Barrier System: Physical and Chemical Environment (BSC 2005 [DIRS 175083]).

The purpose of this model report is to describe the evolution of the physical and chemical environmental conditions within the waste emplacement drifts of the repository, including the drip shield and waste package surfaces. This report documents the development of a new process-level model, the near-field chemistry (NFC) model, and develops two abstraction models.