The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

Past efforts by the Department of Energy (DOE), the Electric Power Research Institute (EPRI), the Nuclear Regulatory Commission (NRC), and others have provided sufficient technical information to enable the NRC to issue regulatory guidance for implementation of pressurized-water reactor (PWR) burnup credit; however, consideration of only the reactivity change due to the major actinides is recommended in the guidance.

Optimization of energy resources suggests increased fuel residence in reactor cores and hence improved
fission product evaluations are required. For thermal reactors the fission product cross sections in the JEF2.2 and
JEFF3.1 libraries plus new evaluations from WPEC23 are assessed through modelling the CERES experiment in
the DIMPLE reactor. The analysis uses the lattice code WIMS10. Cross sections for 12 nuclides are assessed. The
thermal cross section and low energy resonance data for 147,152Sm and 155Gd are accurate to within 4%. Similar data

U.S. Nuclear Regulatory Commission Interim Staff Guidance 8 (ISG-8) for burnup credit covers actinides only, a position based primarily on the lack of definitive critical experiments and adequate radiochemical assay data that can be used to quantify the uncertainty associated with fission product credit.

The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

Target accuracy on LWR neutronics parameters is 2 to 5 times lower than the a priori uncertainty (1σ)
due to nuclear data. This paper summarizes the experimental facilities and the integral measurements that are required
for code qualification. The rigorous use of integral information through trend analysis method is described. Trends
on JEF2 data from Keff measurements and P.I.Es are presented. These trends were accounted for in the new JEFF3
evaluations. The role of fundamental experiments, such as worth measurement of separated isotopes, is emphasized.

Performance objectives for the geologic repository operations area through permanent closure in 10 CFR 63.111 identify compliance with regulatory dose limits for workers and members of the public as a design objective. The purpose of this design calculation is to determine direct radiation dose consequences for Category 1 and 2 event sequences. It does not include worker dose assessment for recovery operations following Category 1 event sequences.