The purpose of this study is to evaluate dissolved concentration limits (also referred to as solubility limits) of elements with radioactive isotopes under probable repository conditions, based on geochemical modeling calculations using geochemical modeling tools, thermodynamic databases, field measurements, and laboratory experiments.

Past efforts by the Department of Energy (DOE), the Electric Power Research Institute (EPRI), the Nuclear Regulatory Commission (NRC), and others have provided sufficient technical information to enable the NRC to issue regulatory guidance for implementation of pressurized-water reactor (PWR) burnup credit; however, consideration of only the reactivity change due to the major actinides is recommended in the guidance.

The purpose of this report is to develop and analyze the Engineered Barrier System (EBS) Radionuclide Transport Abstraction Model, consistent with Level I and Level II model validation, as identified in Technical Work Plan for: Near-Field Environment: Engineered Barrier System: Radionuclide Transport Abstraction Model Report (BSC 2006 [DIRS 177739]). The EBS Radionuclide Transport Abstraction (or RTA) is the conceptual model used in the Total System Performance Assessment (TSPA) to determine the rate of radionuclide releases from the EBS to the unsaturated zone (UZ).

The objective of this calculation is to evaluate the probability of flooding a waste package with seepage water. Disruptive events can affect the Engineered Barrier System (EBS) components and have the potential to allow an advective flow of seepage water to reach the waste package. The advective and diffusive flow paths into the waste package have the potential to result in water accumulation inside the waste package, which in turn can lead to a potentially critical configuration. This calculation will evaluate the following:

Optimization of energy resources suggests increased fuel residence in reactor cores and hence improved
fission product evaluations are required. For thermal reactors the fission product cross sections in the JEF2.2 and
JEFF3.1 libraries plus new evaluations from WPEC23 are assessed through modelling the CERES experiment in
the DIMPLE reactor. The analysis uses the lattice code WIMS10. Cross sections for 12 nuclides are assessed. The
thermal cross section and low energy resonance data for 147,152Sm and 155Gd are accurate to within 4%. Similar data

U.S. Nuclear Regulatory Commission Interim Staff Guidance 8 (ISG-8) for burnup credit covers actinides only, a position based primarily on the lack of definitive critical experiments and adequate radiochemical assay data that can be used to quantify the uncertainty associated with fission product credit.

This study is prepared by the Mined Geologic Disposal System (MODS) Waste Package Development Department (WPDD) to provide input to a separate evaluation on the probablility of criticality in the far- field environment. These calculations are performed in sufficient detail to provide conservatively bounding configurations to support separate probabilistic analyses.

Target accuracy on LWR neutronics parameters is 2 to 5 times lower than the a priori uncertainty (1σ)
due to nuclear data. This paper summarizes the experimental facilities and the integral measurements that are required
for code qualification. The rigorous use of integral information through trend analysis method is described. Trends
on JEF2 data from Keff measurements and P.I.Es are presented. These trends were accounted for in the new JEFF3
evaluations. The role of fundamental experiments, such as worth measurement of separated isotopes, is emphasized.

This report documents the development and validation of the in-drift precipitates/salts (IDPS) process model. The IDPS process model is a geochemical model designed to predict the postclosure effects of evaporation and deliquescence on the chemical composition of water within the Engineered Barrier System (EBS) in support of the total system performance assessment (TSPA). Application of the model in support of TSPA is documented in Engineered Barrier System: Physical and Chemical Environment (BSC 2005 [DIRS 175083]).

The purpose of this model report is to describe the evolution of the physical and chemical environmental conditions within the waste emplacement drifts of the repository, including the drip shield and waste package surfaces. This report documents the development of a new process-level model, the near-field chemistry (NFC) model, and develops two abstraction models.