This analysis provides information necessary for total system performance assessment (TSPA) for the license application (LA) to include the excess U.S. Department of Energy (DOE) plutonium in the form of mixed oxide (MOX) spent nuclear fuel and lanthanide borosilicate (LaBS) glass. This information includes the additional radionuclide inventory due to MOX spent nuclear fuel and LaBS glass and the analysis that shows that the TSPA models for commercial spent nuclear fuel (CSNF) and high-level waste (HLW) degradation are appropriate for MOX spent nuclear fuel and LaBS glass, respectively.

The purpose of this calculation is to develop an estimate of the isotopic content as a function of time for mixed oxide (MOX) spent nuclear fuel (SNF) assemblies in a Westinghouse pressurized water reactor (PWR). These data will be used as source data for criticality, thermal, and radiation shielding evaluations of waste package (WP) designs for MOX assemblies in the Monitored Geologic Repository (MGR).

The "Summary Report of SNF Isotopic Comparisons for the Disposal Criticality Analysis Methodology" contains a summary of the analyses that compare SNF measured isotopic concentrations (radiochemical assays) to calculated SNF isotop~c concentrations (SAS2H module ·orScale4.3). The results of these analyses are used to support the validation of the isotopic models for spent commercial light water reactor (LWR) fuel.

The purpose of this calculation is to document the Crystal River Unit 3 pressurized water reactor (PWR) fuel depletion calculations performed as part of the commercial reactor critical (CRC) evaluation program. The CRC evaluations support the development and validation of the neutronics models used for criticality analyses involving commercial spent nuclear fuel in a geologic repository.

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of the mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.

Taking into account of the loss of reactivity of fuels at the end of their irradiation is known under the
term burnup credit (BUC). It is a question of dimensioning in a less penalizing way the devices of transport,
storage or of processing with respect to the risk of criticality. In the context of nuclear criticality safety a better
realism cannot be obtained at the price of conservatism. As a result the regulator requires measurements make it
possible to validate the adequacy between real fuels and the design assumptions. The sophistication of the

This report presents results from a parametric study of equilibrium fuel cycle costs for a closed fuel cycle with multi-recycling of plutonium in fast reactors (FRs) compared to an open, once-through fuel cycle using PWRs. The study examines the impact on fuel cycle costs from changes in the unit costs of uranium, advanced PUREX reprocessing of discharged uranium dioxide (UO2) fuel and fast-reactor mixed-oxide (FR-MOX) fuel, and FR-MOX fuel fabrication.

Expanding interest in nuclear power and advanced fuel cycles indicate that use of mixed-oxide (MOX) fuel in the current and new U.S. reactor fleet could become an option for utilities in the coming decades. In light of this renewed interest, EPRI has reviewed the substantial knowledge base on MOX fuel irradiation in light water reactors (LWRs). The goal was to evaluate the technical feasibility of MOX fuel use in the U.S. reactor fleet for both existing and advanced LWR designs (Generation III/III+).

Within the context of long-term waste management and sustainable nuclear fuel supply, there continue to be discussions regarding whether the United States should consider recycling of light-water reactor (LWR) spent nuclear fuel (SNF) for the current fleet of U.S. LWRs. This report presents a parametric study of equilibrium fuel cycle costs for an open fuel cycle without plutonium recycling (once-through) and with plutonium recycling (single-recycling using mixed-oxide, or MOX, fuel), assuming an all-pressurized water reactor (PWR) fleet.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
(AFR) criticality safety analyses be validated against experimental measurements. If credit for the
negative reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark AFR criticality analysis methods using selected critical
configurations from commercial pressurized-water reactors (PWR).

STARBUCS is a new prototypic analysis sequence for performing automated criticality safety analyses of spent fuel systems employing burnup credit. A depletion analysis calculation for each of the burnup-dependent regions of a spent fuel assembly, or other system containing spent fuel, is performed using the ORIGEN-ARP sequence of SCALE. The spent fuel compositions are then used to generate resonance self-shielded cross sections for each region of the problem, which are applied in a three-dimensional criticality safety calculation using the KENO V.a code.

As part of the plutonium waste form development and down-select process, repository analyses have been conducted to evaluate the long-term performance of these forms for repository acceptance. Intact and degraded mode criticality analysis of the mixed oxide (MOX) spent fuel is presented in Volume I, while Volume II presents the evaluations of the waste form containing plutonium immobilized in a ceramic matrix.

The purpose of this calculation is to perform a parametric study to determine the effects of fission product leaching, assembly collapse, and iron oxide loss (Me203) on the reactivity of a waste package (WP) containing mixed oxide (MOX) spent nuclear fuel (SNF). Previous calculations (CRWMS M&O 1998a) have shown that the criticality control features of the WP are adequate to prevent criticality of a flooded WP for all the enrichment/ burnup pairs expected for the MOX SNF.

The purpose of this calculation is to perform a parametric study to determine the effects of fission product leaching, assembly collapse, and iron oxide loss on the reactivity of a waste package containing mixed oxide spent nuclear fuel. Previous calculations (CRWMS M&O 1998a) have shown that the criticality control features of the waste package are adequate to prevent criticality of a flooded WP for all the enrichment/burnup pairs expected for the MOX SNF.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

The requirements of ANSI/ANS 8.1 specify that calculational methods for away-from-reactor
criticality safety analyses be validated against experimental measurements. If credit for the negative
reactivity of the depleted (or spent) fuel isotopics is desired, it is necessary to benchmark
computational methods against spent fuel critical configurations. This report summarizes a portion
of the ongoing effort to benchmark away-from-reactor criticality analysis methods using critical
configurations from commercial pressurized-water reactors.

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.

This calculation file provides comparisons of one- and two-dimensional methods for calculating the isotopic content of spent nuclear fuel. The one-dimensional methods use the SAS2H sequence of SCALE 4.4a (Reference 7.1) and the SAS2 sequence of SCALE 5.0 (Reference 7.2). The two-dimensional method uses the TRITON control module along with the T-DEPL sequence of SCALE 5.0 (Reference 7.3). The SAS2H results for SCALE 4.4a are taken from Reference 7.4. Data from previous two-dimensional calculations (Reference 7.5) using CASM03 will also be used for comparisons with TRITON.

Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been
modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system.
The SAS2H sequence uses transport methods combined with the depletion and decay capabilities
of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup
history. Results of these calculations are compared with chemical assay measurements of spent fuel
inventories for each sample. Results show reasonable agreement between measured and predicted

Disposal Criticality Analysis Methodology Topical Report describes a methodology for performing postclosure criticality analyses within the repository at Yucca Mountain, Nevada. An important component of the postclosure criticality analysis is the calculation of conservative isotopic concentrations for spent nuclear fuel. This report documents the isotopic calculation methodology. The isotopic calculation methodology is shown to be conservative based upon current data for pressurized water reactor and boiling water reactor spent nuclear fuel.

The purpose of this calculation is to perform criticality evaluations for mixed oxide spent nuclear fuel (MOX SNF) in 12 and 21 Pressurized Water Reactor (PWR) waste packages (WPs) for both intact and degraded configurations.
The MOX assembly design considered in previous studies on Pu disposition in commercial reactors is based on the Westinghouse (W) 17x17 Vantage 5 assembly (Ref. 7.2). Depletion analyses of four Pu enrichment and burnup (expressed as gigawatt days/metric ton heavy metal; GWd/MTHM) combinations were performed in Reference 7.4. These are:

The purpose of this design analysis is to determine the accuracy of the SAS2H module of SCALE 4.3 in predicting isotopic concentrations of spent fuel assemblies. The objective is to develop a methodology for modeling assemblies similar to those evaluated within this analysis and to establish the consistency of SAS2H predictions. The results of this analysis may then be applied to future depletion calculations using SAS2H in which no measurements are available.