The preclosure criticality analysis process described in this technical report provides a systematic approach for determining the need for criticality controls and for evaluating their effectiveness during the preclosure period of the Monitored Geologic Repository at Yucca Mountain, Nevada.

The Monitored Geologic Repository (MGR) Waste Package Operations (WPO) of the Civilian Radioactive Waste Management System Management and Operating Contractor (CRWMS M&O) performed calculations to provide input for disposal of Pu-ceramic waste forms. The Pu- ceramic (Refs. 1 and 2) is designed to immobilize excess plutonium from weapons production, and has been considered for disposal at the potential Yucca Mountain site.

This “Technical Evaluation Report on the Content of the U.S. Department of Energy’s Yucca Mountain License Application; Postclosure Volume: Repository Safety After Permanent Closure” (TER Postclosure Volume) presents information on the NRC staff’s review of DOE’s Safety Analysis Report (SAR), provided on June 3, 2008, as updated by DOE on February 19, 2009. The NRC staff also reviewed information DOE provided in response to NRC staff’s requests for additional information and other information that DOE provided related to the SAR.

The purpose of this calculation is to apply the process described in the TDR-DS0-NU-000001 Rev. 02, Preclosure Criticality Analysis Process Report (Ref. 2.2.25) to aid in establishing design and operational criteria important to criticality safety and to identify potential control parameters and their limits important to the criticality safety of commercial spent nuclear fuel (CSNF) handling operations in the Wet Handling Facility (WHF)

This analysis provides information necessary for total system performance assessment (TSPA) for the license application (LA) to include the excess U.S. Department of Energy (DOE) plutonium in the form of mixed oxide (MOX) spent nuclear fuel and lanthanide borosilicate (LaBS) glass. This information includes the additional radionuclide inventory due to MOX spent nuclear fuel and LaBS glass and the analysis that shows that the TSPA models for commercial spent nuclear fuel (CSNF) and high-level waste (HLW) degradation are appropriate for MOX spent nuclear fuel and LaBS glass, respectively.

The purpose of this scientific analysis is to document the results and interpretations of field experiments that test and validate conceptual flow and radionuclide transport models in the saturated zone (SZ) near Yucca Mountain, Nevada. The test interpretations provide estimates of flow and transport parameters used in the development of parameter distributions for total system performance assessment (TSPA) calculations.

This analysis is prepared by the Mined Geologic Disposal System (MGDS) Waste Package Development Department (WPDD) to provide an assessment of the present waste package design from a criticality risk standpoint. The specific objectives of this initial analysis are to:
1. Establish a process for determining the probability of waste package criticality as a function of time (in terms of a cumulative distribution function, probability distribution function, or expected number of criticalities in a specified time interval) for various waste package concepts;

Letter from the Congress of the United States House of Representatives, Committee on Energy and Commerce.

The Disposal Criticality Analysis Methodology Topical Report (YMP 2003) presents the methodology for evaluating potential criticality situations in the monitored geologic repository. As stated in the referenced Topical Report, the detailed methodology for performing the disposal criticality analyses will be documented in model reports. Many of the models developed in support of the Topical Report differ from the definition of models as given in the Office of Civilian Radioactive Waste Management procedure AP-SIII.10Q, Models, in that they are procedural, rather than mathematical.

The success of the Civilian Radioactive Waste Management Program of the U.S.
Department of Energy (DOE) is critical to U.S. ability to manage and dispose of
nuclear waste safely--and to the reestablishment of confidence in the nuclear energy
option in the United States. The program must conform with all applicable standards
and, in fact, set the example for a national policy on the safe disposal of radioactive
waste.
The Secretary of Energy has recently completed an extensive review of the

By the end of this century, the United States plans to begin operating the first geologic repository for the permanent disposal of commercial spent nuclear fuel and high-level radioactive Waste. Public Law 97-425, the Nuclear waste Policy Act of 1982 (the Act), specifies the process for selecting a repository site, and constructing, operating, closing, and decommissioning the repository.

This analysis is prepared by the Mined Geologic Disposal System (MGDS) Waste Package Development (WPD) department to provide a probabilistic evaluation of the potential for criticality of fissile material which has been transported from a geologic repository containing breached waste packages of commercial spent nuclear fuel (SNF). This analysis is part of a continuing investigation of the probability of criticality resulting from the emplacement of spent nuclear fuel in a geologic repository.

This report presents the results of computer code benchmark simulations against spent fuel radiochemical assay
measurements from the Kansai Electric Ltd. Takahama-3 reactor published by the Japan Atomic Energy
Research Institute. Takahama-3 is a pressurized-water reactor that operates with a 17 × 17 fuel-assembly design.
Spent fuel samples were obtained from assemblies operated for 2 and 3 cycles and achieved a maximum burnup
of 47 GWd/MTU. Radiochemical analyses were performed on two rods having an initial enrichment of